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H-bonding dependent phosphorescence in a mixed ligand copper(I) complex

Articolo
Data di Pubblicazione:
2018
Abstract:
The mixed ligand copper(I) derivative [Cu(PPh3)2(j2-O,O00-lact)] (1) (lact = L-(+)-lactate) has been prepared
and fully characterized. NMR studies indicated the occurrence of a fluxional behavior involving
the lactate anion, in solution. The a-hydroxycarboxylate ligand is responsible for the generation of a catemeric
O–H O(CO) H-bonding network that strongly influences the photophysical properties of 1, in the
solid state. Indeed, when irradiated with UV light the title compound shows a bright phosphorescence,
which as suggested by DFT calculations is strictly related to the abovementioned H-bonding network.
Tipologia CRIS:
Articolo su Rivista
Keywords:
Copper(I) Hydrogen bonds Phosphorescence Lactate a-Hydroxycarboxylates
Elenco autori:
Durini, S.; Ardizzoia, G. A.; Colombo, Gioele; Therrien, B.; Brenna, S.
Autori di Ateneo:
ARDIZZOIA GIAN ATTILIO
BRENNA STEFANO
COLOMBO GIOELE
Link alla scheda completa:
https://irinsubria.uninsubria.it/handle/11383/2066399
Pubblicato in:
POLYHEDRON
Journal
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http://www.journals.elsevier.com/polyhedron/
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